Misra, Sambuddha; Froelich, Philip N. (2012): Lithium isotope history of Cenozoic seawater; changes in silicate weathering and reverse weathering. American Association for the Advancement of Science, Washington, DC, United States, Science, 335 (6070), 818-823, georefid:2012-037638

Abstract:
Weathering of uplifted continental rocks consumes carbon dioxide and transports cations to the oceans, thereby playing a critical role in controlling both seawater chemistry and climate. However, there are few archives of seawater chemical change that reveal shifts in global tectonic forces connecting Earth ocean-climate processes. We present a 68-million-year record of lithium isotopes in seawater (delta (super 7) Li (sub SW) ) reconstructed from planktonic foraminifera. From the Paleocene (60 million years ago) to the present, delta (super 7) Li (sub SW) rose by 9 ppm, requiring large changes in continental weathering and seafloor reverse weathering that are consistent with increased tectonic uplift, more rapid continental denudation, increasingly incongruent continental weathering (lower chemical weathering intensity), and more rapid CO (sub 2) drawdown. A 5ppm drop in delta (super 7) Li (sub SW) across the Cretaceous-Paleogene boundary cannot be produced by an impactor or by Deccan trap volcanism, suggesting large-scale continental denudation.
Coverage:
West: -46.0000 East: 92.0000 North: 8.0000 South: -40.0000
West: NaN East: NaN North: NaN South: NaN
West: NaN East: NaN North: NaN South: NaN
West: NaN East: NaN North: NaN South: NaN
Relations:
Expedition: 121
Site: 121-757
Site: 121-758
Expedition: 154
Site: 154-926
Expedition: 208
Site: 208-1262
Site: 208-1263
Site: 208-1265
Site: 208-1267
Supplemental Information:
Supplemental information/data is available in the online version of this article; related article by Paytan, A., on p. 810-811
Data access:
Provider: SEDIS Publication Catalogue
Data set link: http://sedis.iodp.org/pub-catalogue/index.php?id=10.1126/science.1214697 (c.f. for more detailed metadata)
Data download: application/pdf
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